If you noticed I'm posting the Bonds in order but backwards and I'm going now with the classic actors. Roger Moore still is one of the most famous Bond actors and did the unthinkable and give the character a major boost in popularity following the excellence of Sean Connery. Sure his films were campy but what he added to the character in terms of personality outweighed anything camp. His Bond was laid back, overconfident, charming funny and a womanizer machine. It's still a blast seeing him play the character. He even beat Connery with total films as Bond with 7 (Connery did 6)
If someone would jump over crocodiles like an expert Super Mario that's Moore, Roger Moore.